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The reactions of PINO • with substituted toluenes, benzaldehydes, and benzyl alcohols were investigated under an argon atmosphere. 
The reactions with toluenes and benzyl alcohols have better correlations with σ + (ρ = −1.3 and −0.41), and the reaction with benzaldehydes correlates better with σ (ρ = −0.91). The second-order rate constants were correlated by means of a Hammett analysis.
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